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Preparation of catalyst coated membranes using screen printing

Includes abstract.

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Main Author: Hill, Matthew Raymond
Other Authors: Conrad, Olaf
Format: Thesis
Language:English
Published: Department of Chemical Engineering 2015
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access_status_str Open Access
author Hill, Matthew Raymond
author2 Conrad, Olaf
author_browse Conrad, Olaf
Hill, Matthew Raymond
author_facet Conrad, Olaf
Hill, Matthew Raymond
author_sort Hill, Matthew Raymond
collection Thesis
description Includes abstract.
format Thesis
id oai:open.uct.ac.za:11427/11834
institution University of Cape Town (South Africa)
language eng
last_indexed 2026-06-10T12:46:23.416Z
license_str Not specified — see source repository
provenance_str_mv Harvested via OAI-PMH from UCTD — University of Cape Town Open Access Repository
publishDate 2015
publishDateRange 2015
publishDateSort 2015
publisher Department of Chemical Engineering
publisherStr Department of Chemical Engineering
record_format dspace
source_str UCTD — University of Cape Town Open Access Repository
spelling oai:open.uct.ac.za:11427/11834 Preparation of catalyst coated membranes using screen printing Hill, Matthew Raymond Conrad, Olaf Engineering Includes abstract. Includes bibliographical references. Of the various types of fuel cells, Polymer Electrolyte Fuel Cells (PEFCs) have already been demonstrated in transportation appliances from light-duty vehicles to buses and in portable appliances including laptops and cell phones. A key component of a PEFC is its platinum electrocatalyst. With an estimated 75% of the world’s platinum reserves and resources in South Africa, local development of this technology will allow South Africa to become a major player in the growing hydrogen economy. This project therefore forms part of the Department of Science and Technologies strategy, to develop fuel cell technology in South Africa. More specifically, this study aims to contribute to the development of membrane electrode assembly (MEA) platform technology at the HySA/Catalysis Centre. In order to achieve this goal, a catalyst coated membrane (CCM) fabrication procedure was implemented using a newly acquired screen printer. In this procedure, catalyst ink is forced through a mesh onto a substrate, where it can then be transferred to a membrane via decal transfer to form a CCM. Two gas diffusions layers can then be placed on either side of the CCM forming a 5-layered MEA. Characterisation techniques of the catalyst ink, CCM and 5-layered MEA were successfully implemented such that future researchers can expand on the ideas. Catalyst inks with varying amounts of isopropanol, 1,2-propanediol and water were screened for their suitability for screen printing. In particular the catalyst ink rheology required for a smooth and even printed surface was determined for a given screen and squeegee combination. With all the established steps in pace, screen printing proved to be a fast and reliable approach for CCM fabrication with potential for future scale up and commercialisation. The fabricated CCMs performed on a par with a commercial Ion Power CCM, but under performed in comparison to a commercial Johnson Matthey (JM) MEA. Possible reasons for this include improved materials in the JM MEA and cell conditions favouring the JM MEA. Future projects which specifically arise from this work entail an investigation into the water management of the fuel cell environment at HySA/Catalysis, as well as a modification of the various steps in order to optimise the process and in doing so manufacture commercially viable MEAs. 2015-01-09T08:56:31Z 2015-01-09T08:56:31Z 2013 Master Thesis Masters MSc http://hdl.handle.net/11427/11834 eng application/pdf Department of Chemical Engineering Faculty of Engineering and the Built Environment University of Cape Town
spellingShingle Engineering
Hill, Matthew Raymond
Preparation of catalyst coated membranes using screen printing
thesis_degree_str Master's
title Preparation of catalyst coated membranes using screen printing
title_full Preparation of catalyst coated membranes using screen printing
title_fullStr Preparation of catalyst coated membranes using screen printing
title_full_unstemmed Preparation of catalyst coated membranes using screen printing
title_short Preparation of catalyst coated membranes using screen printing
title_sort preparation of catalyst coated membranes using screen printing
topic Engineering
url http://hdl.handle.net/11427/11834
work_keys_str_mv AT hillmatthewraymond preparationofcatalystcoatedmembranesusingscreenprinting