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Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium

In the experimental determination of the half-life of the decay of a radioactive element, an aluminium cylinder is activated through immersion in a thermal neutron bath. The decay of the irradiated aluminium cylinder is then measured to determine the half-life of the resultant 28Al. During the execu...

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Main Author: Nel, Andre Pierre
Other Authors: Aschman, David
Format: Thesis
Language:English
Published: Department of Electrical Engineering 2019
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access_status_str Open Access
author Nel, Andre Pierre
author2 Aschman, David
author_browse Aschman, David
Nel, Andre Pierre
author_facet Aschman, David
Nel, Andre Pierre
author_sort Nel, Andre Pierre
collection Thesis
description In the experimental determination of the half-life of the decay of a radioactive element, an aluminium cylinder is activated through immersion in a thermal neutron bath. The decay of the irradiated aluminium cylinder is then measured to determine the half-life of the resultant 28Al. During the execution of the experiment, unsuspected gamma ray peaks other than the expected 1.78 MeV from the decay of the activated 28Al are however observed. Two potential hypotheses are considered in the study. The first hypothesis is that the 27Al from which the aluminium cylinder is manufactured is not pure and contains certain impurities which could be activated resulting in the measurement of the decay of materials other than the intended 28Al. The second hypothesis is the inadequate moderation of the neutrons resulting in the interaction of fast neutrons with the aluminium cylinder and hence the creation of something other than the intended 28Al. Based on the results of the two experiments conducted, it has been demonstrated that there is some evidence, though not very convincing, that both postulated hypotheses potentially hold true. Considering the relatively small amounts of alloying elements in a typical aluminium sample and the poor correlation between published half-lives with the derived half-lives from the experiment, the hypothesis that the impurities in the aluminium from which the aluminium cylinder is manufactured are activated when immersed in the neutron bath resulting in the measurement of the decay of materials other than the intended 28Al, is considered possible but improbable. On the other hand, considering the pertinence of the decay signature of 27Mg in both experiments, the observed increase in the 27Mg activity in the unmoderated activation, the abundance of the target nuclei of 27Al, as well as the increase in the 27Al (n,p) 27Mg reaction with increased neutron energy, hypotheses 2 is deemed both possible and probable.
format Thesis
id oai:open.uct.ac.za:11427/30035
institution University of Cape Town (South Africa)
language eng
last_indexed 2026-06-10T12:53:10.288Z
license_str Not specified — see source repository
provenance_str_mv Harvested via OAI-PMH from UCTD — University of Cape Town Open Access Repository
publishDate 2019
publishDateRange 2019
publishDateSort 2019
publisher Department of Electrical Engineering
publisherStr Department of Electrical Engineering
record_format dspace
source_str UCTD — University of Cape Town Open Access Repository
spelling oai:open.uct.ac.za:11427/30035 Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium Nel, Andre Pierre Aschman, David In the experimental determination of the half-life of the decay of a radioactive element, an aluminium cylinder is activated through immersion in a thermal neutron bath. The decay of the irradiated aluminium cylinder is then measured to determine the half-life of the resultant 28Al. During the execution of the experiment, unsuspected gamma ray peaks other than the expected 1.78 MeV from the decay of the activated 28Al are however observed. Two potential hypotheses are considered in the study. The first hypothesis is that the 27Al from which the aluminium cylinder is manufactured is not pure and contains certain impurities which could be activated resulting in the measurement of the decay of materials other than the intended 28Al. The second hypothesis is the inadequate moderation of the neutrons resulting in the interaction of fast neutrons with the aluminium cylinder and hence the creation of something other than the intended 28Al. Based on the results of the two experiments conducted, it has been demonstrated that there is some evidence, though not very convincing, that both postulated hypotheses potentially hold true. Considering the relatively small amounts of alloying elements in a typical aluminium sample and the poor correlation between published half-lives with the derived half-lives from the experiment, the hypothesis that the impurities in the aluminium from which the aluminium cylinder is manufactured are activated when immersed in the neutron bath resulting in the measurement of the decay of materials other than the intended 28Al, is considered possible but improbable. On the other hand, considering the pertinence of the decay signature of 27Mg in both experiments, the observed increase in the 27Mg activity in the unmoderated activation, the abundance of the target nuclei of 27Al, as well as the increase in the 27Al (n,p) 27Mg reaction with increased neutron energy, hypotheses 2 is deemed both possible and probable. 2019-05-10T11:49:45Z 2019-05-10T11:49:45Z 2018 2019-05-07T11:27:58Z Master Thesis Masters MSc (Eng) http://hdl.handle.net/11427/30035 eng application/pdf Department of Electrical Engineering Faculty of Engineering and the Built Environment
spellingShingle Nel, Andre Pierre
Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium
thesis_degree_str Master's
title Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium
title_full Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium
title_fullStr Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium
title_full_unstemmed Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium
title_short Study of unsuspected gamma ray energy peaks observed during the determination of the half-life of activated aluminium
title_sort study of unsuspected gamma ray energy peaks observed during the determination of the half life of activated aluminium
url http://hdl.handle.net/11427/30035
work_keys_str_mv AT nelandrepierre studyofunsuspectedgammarayenergypeaksobservedduringthedeterminationofthehalflifeofactivatedaluminium