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Determining non-linear optical properties using the Z-scan technique

Thesis (MSc (Physics))--University of Stellenbosch, 2005.

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Main Author: Neethling, Pieter H.
Other Authors: Rohwer, Erich G.
Format: Thesis
Language:English
Published: Stellenbosch : University of Stellenbosch 2008
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access_status_str Open Access
author Neethling, Pieter H.
author2 Rohwer, Erich G.
author_browse Neethling, Pieter H.
Rohwer, Erich G.
author_facet Rohwer, Erich G.
Neethling, Pieter H.
author_sort Neethling, Pieter H.
collection Thesis
dc_rights_str_mv University of Stellenbosch
description Thesis (MSc (Physics))--University of Stellenbosch, 2005.
format Thesis
id oai:scholar.sun.ac.za:10019.1/2094
institution Stellenbosch University (South Africa)
language English
last_indexed 2026-06-10T12:41:45.229Z
license_str Other — see source repository
provenance_str_mv Harvested via OAI-PMH from SUNScholar — Stellenbosch University Repository
publishDate 2008
publishDateRange 2008
publishDateSort 2008
publisher Stellenbosch : University of Stellenbosch
publisherStr Stellenbosch : University of Stellenbosch
record_format dspace
source_str SUNScholar — Stellenbosch University Repository
spelling oai:scholar.sun.ac.za:10019.1/2094 Determining non-linear optical properties using the Z-scan technique Neethling, Pieter H. Rohwer, Erich G. University of Stellenbosch. Faculty of Science. Dept. of Physics. Nonlinear optics Optical scanners Scanning systems Dissertations -- Physics Theses -- Physics Thesis (MSc (Physics))--University of Stellenbosch, 2005. The extremely high light intensities produced by lasers and the increasing use of lasers highlights the need for measures to prevent damage to materials due to exposure to high intensity laser light. In particular it necessitates the development of systems to protect optical sensors, including the human eye. In this work optical limiters were investigated as a system for protecting sensors. An optical limiter transmits ambient light, but absorbs high intensity light. This makes it ideal for protecting sensors from laser radiation, since it allows the sensor to operate unhindered at design intensities while protecting it from harmful high intensity radiation. There are various mechanisms used for optical limiting, and in this work the nonlinear absorption and the nonlinear index of refraction changes of materials were investigated. A facility was established to measure the nonlinear optical properties of a variety of materials, in order to classify them as possible optical limiters. This entailed creating a so called Zscan setup, which enabled us to measure the nonlinear absorption coefficient and the nonlinear index of refraction of a material. The theory and the design of the setup are discussed and experimental results obtained using this setup are presented. A wide variety of material types were investigated to show the versatility of the experimental setup. These included C60, which was analyzed in solution; ZnO which is a crystal; CdS quantum dots in solution; and poly(dioctyl-fluorene), which is a large polymer molecule, in solution. The materials investigated in this work were chosen based on their known strong nonlinear optical properties. Emphasis was placed on measuring the nonlinear absorption coefficients since it was the dominant optical limiting effect of the materials under investigation. The results obtained displayed the same trends as published results and it shows that the established facility was capable of measuring the nonlinear properties of these samples. The experimental limitations of the setup were determined, and critical experimental parameters were identified for measurements of this nature. Improvements to the experimental facility are suggested to improve the accuracy of future measurements. 2008-07-22T12:50:46Z 2010-06-01T08:40:22Z 2008-07-22T12:50:46Z 2010-06-01T08:40:22Z 2005-03 Thesis http://hdl.handle.net/10019.1/2094 en University of Stellenbosch application/pdf Stellenbosch : University of Stellenbosch
spellingShingle Nonlinear optics
Optical scanners
Scanning systems
Dissertations -- Physics
Theses -- Physics
Neethling, Pieter H.
Determining non-linear optical properties using the Z-scan technique
title Determining non-linear optical properties using the Z-scan technique
title_full Determining non-linear optical properties using the Z-scan technique
title_fullStr Determining non-linear optical properties using the Z-scan technique
title_full_unstemmed Determining non-linear optical properties using the Z-scan technique
title_short Determining non-linear optical properties using the Z-scan technique
title_sort determining non linear optical properties using the z scan technique
topic Nonlinear optics
Optical scanners
Scanning systems
Dissertations -- Physics
Theses -- Physics
url http://hdl.handle.net/10019.1/2094
work_keys_str_mv AT neethlingpieterh determiningnonlinearopticalpropertiesusingthezscantechnique