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The production of 139Pr and 139Ce in proton-induced reactions

Thesis (MSc (Chemistry and Polymer Science))--University of Stellenbosch, 2007.

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Main Author: Vermeulen, Christiaan
Other Authors: Steyn, G. F.
Format: Thesis
Language:en_ZA
Published: Stellenbosch : University of Stellenbosch 2008
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access_status_str Open Access
author Vermeulen, Christiaan
author2 Steyn, G. F.
author_browse Steyn, G. F.
Vermeulen, Christiaan
author_facet Steyn, G. F.
Vermeulen, Christiaan
author_sort Vermeulen, Christiaan
collection Thesis
dc_rights_str_mv University of Stellenbosch
description Thesis (MSc (Chemistry and Polymer Science))--University of Stellenbosch, 2007.
format Thesis
id oai:scholar.sun.ac.za:10019.1/2130
institution Stellenbosch University (South Africa)
language en_ZA
last_indexed 2026-06-10T12:44:25.612Z
license_str Other — see source repository
provenance_str_mv Harvested via OAI-PMH from SUNScholar — Stellenbosch University Repository
publishDate 2008
publishDateRange 2008
publishDateSort 2008
publisher Stellenbosch : University of Stellenbosch
publisherStr Stellenbosch : University of Stellenbosch
record_format dspace
source_str SUNScholar — Stellenbosch University Repository
spelling oai:scholar.sun.ac.za:10019.1/2130 The production of 139Pr and 139Ce in proton-induced reactions Vermeulen, Christiaan Steyn, G. F. University of Stellenbosch. Faculty of Science. Dept. of Chemistry and Polymer Science. Radioisotopes Isotope separation Dissertations -- Chemistry Theses -- Chemistry Thesis (MSc (Chemistry and Polymer Science))--University of Stellenbosch, 2007. Excitation functions and production rates are presented for various Ce and Pr radionuclides formed in the bombardment of 141Pr, natLa and natCe with protons. Extensive measure- ments were performed for 141Pr + p up to 100 MeV and for natLa + p up to 20 MeV. The possibility is investigated to utilize tandem targetry for the production of no-carrier-added 139Ce of high radionuclidic purity, having a Pr target in the higher energy slot followed by a La target in a lower energy slot. 141Pr(p,3n)139mNd!139Pr is investigated as an al- ternative to the direct production route 140Ce(p,2n)139Pr for producing no-carrier-added 139Pr of high radionuclidic purity. The advantages and disadvantages of both production routes are discussed. The simultaneous production of 139Pr and 140Nd using Pr as target is also investigated. Experimental thick-target production rates are presented for Pr ra- dionuclides formed in the bombardment of natCe with protons at incident energies of 20, 26 and 32 MeV. All the experimental excitation functions obtained in this work are compared with theoretical predictions by means of the geometry-dependent hybrid (GDH) model as implemented in the code ALICE-IPPE. The results of this work are also compared with previous literature experimental data, if available. 2008-04-14T13:41:41Z 2010-06-01T08:41:03Z 2008-04-14T13:41:41Z 2010-06-01T08:41:03Z 2007-12 Thesis http://hdl.handle.net/10019.1/2130 en_ZA University of Stellenbosch 4544872 bytes application/pdf application/pdf Stellenbosch : University of Stellenbosch
spellingShingle Radioisotopes
Isotope separation
Dissertations -- Chemistry
Theses -- Chemistry
Vermeulen, Christiaan
The production of 139Pr and 139Ce in proton-induced reactions
title The production of 139Pr and 139Ce in proton-induced reactions
title_full The production of 139Pr and 139Ce in proton-induced reactions
title_fullStr The production of 139Pr and 139Ce in proton-induced reactions
title_full_unstemmed The production of 139Pr and 139Ce in proton-induced reactions
title_short The production of 139Pr and 139Ce in proton-induced reactions
title_sort production of 139pr and 139ce in proton induced reactions
topic Radioisotopes
Isotope separation
Dissertations -- Chemistry
Theses -- Chemistry
url http://hdl.handle.net/10019.1/2130
work_keys_str_mv AT vermeulenchristiaan theproductionof139prand139ceinprotoninducedreactions
AT vermeulenchristiaan productionof139prand139ceinprotoninducedreactions